This is a pretty good idea. I tend to use the hollow rock outside of Megaton for early storage, and this is far better. I'd prefer a locker or something Megaton-ish rather than an Enclave crate, but that's just me. You might consider enabling the key only after the player has agreed to begin Moira's Wasteland Survival guide quest, granting the storage as side benefit of working with her.
Hollow rock along the right outer wall of Megaton, near some Mole Rats, wedged between three small trees. It contains a strong gun for early on in the game.
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I have no plans on playing Fallout 3 again.
<Should have to pay Moira about 100 caps per week tho, but that's plenty of time to defuse the bomb and get the vanilla player house>
The lockers in the common room were annoying to get to.
Have Fun!